i think Big O is pretty cool. check out Paranoia Agent. gets interesting and if you havent checked out all the Miyazaki films, you must.
Akira is the only anime movie I've seen in its entirety so its my favorite. The final chapter/part of the animatrix was pretty cool and really trippy.
Favorite show is definitely Rurouni Kenshin, Noein, or Gundam Wing Movie is either Princess Mononoke, Spirited Away, Howl's Moving Castle, or Paprika
Gungrave and Venus Versus Virus are becoming my recent favs. I'm trying to find some Witchblade and Claymore, though cause I demoed them on my girlfriend's netflix and they looked pretty badass. Same with Blood
Yeah, I found witchblade there (yesterday) but it took like 23 hours to download. Pretty HQ though, and I'm not a snob at all. So far I found blood, claymore, witchblade and like everything else ever on ani4free.com though, all hosted on mediafire... so that's definitely the route for me from now on.